Marie Harf, a State Department spokeswoman, said Kerry spoke Monday with his British, Jordanian, Qatari and Saudi counterparts, as well as the secretary-general of the Arab League.
The diplomatic efforts appeared to be working, with an Arab League spokesman condemning the al-Assad regime Tuesday for the chemical attack.
In another move, the United States postponed its involvement in talks scheduled for this week in Geneva on seeking a political solution to the Syrian civil war. Russia expressed disappointment at the U.S. decision and warned against any Western military strike on Syria.
Last month, Joint Chiefs Chairman Gen. Martin Dempsey provided Congress with a list of declassified U.S. military options for Syria that emphasized the high costs and risks of what he said would amount to "an act of war" at a time of deep budget cuts.
Dempsey's letter, dated July 19, listed U.S. assets in the region including Patriot missile defense batteries in Turkey and Jordan, as well as F-16 jet fighters positioned to defend Jordan from possible cross-border trouble. In addition, the Pentagon has sent four warships armed with cruise missiles to the region.
According to U.S. officials, updated options offered to the president in recent days included:
• Cruise missiles fired from one of four Navy destroyers deployed in the Mediterranean Sea. The missiles would be used to strike "command and control" facilities such as command bunkers, or the Syrian regime's means of delivering chemical weapons: artillery batteries and launchers. There is no indication that the missiles would strike actual chemical weapons stockpiles.
• Military jets firings weapons from outside Syrian airspace. This option carries additional risks and is considered less likely.
To Aaron David Miller, a vice president at the Woodrow Wilson International Center, the situation is forcing Obama to shift from being an "avoider-in-chief" regarding military involvement in Syria.
"It's almost inevitable that the president will authorize some form of military action," Miller told National Public Radio in an interview broadcast Monday.
He said he expected a significant response that amounts to "a warning that lays down this time a red line that the president intends to enforce, not one that turns pink."
"It cannot simply be a couple of cruise missiles into a storage shed somewhere," Miller said, adding that the goal was to deter al-Assad rather than topple him or radically shift the balance in Syria at this time. "The president's not on the verge of becoming the cavalry to rescue the country."